Yuri is incredible in the role but it's too subjective to crown any one Actor as the absolute best just due to the different variables in all the iterations of Spider Man. There's Peter/Spidey in his Teens, 20's, and 30's and all of them are at such different points in their lives due to experiences that the nuances in the characters make the portrayal. And that's before considering the context of each of these time periods of Peter's life being contemporary to the time they were made. I.E. Tobey's "teen" Peter and Holland's "teen" Peter were always going to be very different due to the way the world was at the time the movies were made.
But if I had to pick, I'd say Holland is the best Teenage Peter/Spidey, Yuri the best 20's, and Jake Johnson the best 30's. All of their portrayals are great and ring true to the character in the context of time period.